The main reason I want to overclock anything is because I'm running dual GTX 580s in SLI, and feel like I'm missing out on performance. I recently fixed a large part of my problem by disabling HTEP and Hyperthreading in the BIOS, but I'm still reading around Battlelog and the NVIDIA forums that other users are averaging in the 80-120 range constant, where there are times when my frame rate dips into the 50s (a rare occurrence, but it happens nonetheless).
I was able to overclock by i7 950 to over 3.8 GHz, but noticed a -decrease- in performance with VSync enabled. I'm not sure if I even overclocked it properly, since all I did was edit values in the BIOS until my CPU host frequency was 3800+ MHz. I tried upping the voltage (didn't know how, or what, to adjust), and ended up having to reset the CMOS via removing the battery. I'm running stock right now, since the performance I was getting before trying to overclock was fine, I was just curious as to how other seemingly identical systems can destroy Battlefield 3, where I only come close.
Edit: What I would like to see is a constant frame rate above 60. Anything below 60 I can tell the difference, and it affects my gameplay. If I can maintain a steady 60 frames per second no matter what I'm looking at, I'm happy.